Synonyms of unnerve in English:
the bleakness of his gaze unnerved her
demoralize, discourage, dishearten, dispirit, deject, daunt, cow, alarm, frighten, unman, dismay, distress, disconcert, discompose, perturb, upset, discomfit, take aback, unsettle, disquiet, jolt, startle, fluster, agitate, shake, ruffle, throw, throw off balance, put someone off their stroke, cause someone to lose their composure, confound, panic, stupefy, stun
British informalput the wind up
[Antonyms] encourage, hearten
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